As the major absorbing aerosols, black carbon (BC) exerts positive radiative forcing on the atmosphere and affects the radiation balance of the earth-atmosphere system and hence aerosol-boundary interactions. Although air quality in the megacity of Beijing has been improved significantly since the implementation of the Clean Air Action Plan in 2013, the long-term changes in BC and optical properties of aerosols are poorly known, let alone their impacts.

A photo of haze over Beijing. Also shown are the instruments of four-cup anemometers, meteoprobe, ultrasonic anemometer and visibility meter installed on the Beijing 325 m meteorological tower. (Image by LI Hao)

Professor SUN Yele and his team from the Institute of Atmospheric Physics, Chinese Academy of Sciences conducted nine-year measurements of BC and light extinction coefficient in Beijing from 2012 to 2020. By analysing the long-term changes in BC, single-scattering albedo (SSA), mass extinction efficient (MEE), brown carbon (BrC) and absorption Angstrom exponent, they demonstrated the response of BC and optical properties to the Clean Air Action Plan, and evaluated the impacts of BC and BrC on direct radiative forcing.

This study was published in Atmospheric Chemistry and Physics.

"The BC decreased by approximately 71% during the last decade in Beijing and the decreases were different in different seasons." said Prof. SUN, "We found that BC showed the most significant reductions in autumn and at night due to the decreased emissions in biomass burning and heavy-duty vehicles".

"The particle extinction coefficient that is directly related to visibility also decreased by 47%. Our results supported that the Clean Air Action Plan has been a great success in mitigating air pollution in Beijing", said Prof. SUN, "However, we found that the different changes in BC and extinction coefficient have caused the increases in SSA and MEE. That is, scattering aerosols are more important in affecting aerosol radiative forcing". Prof. SUN continued to say, "The increased MEE might not be a good sign because it will bring new challenges to improve atmospheric visibility in Beijing in the future."

According to Prof. SUN's study, the changes in BC, BrC and aerosol optical properties have significant implications in changing their radiative effects and aerosol-boundary layer interactions. Future mitigation of air pollution in megacities need to take these changes into account.

Reference:
Sun, J., Wang, Z., Zhou, W., Xie, C., Wu, C., Chen, C., Han, T., Wang, Q., Li, Z., Li, J., Fu, P., Wang, Z., and Sun, Y.: Measurement report: Long-term changes in black carbon and aerosol optical properties from 2012 to 2020 in Beijing, China, Atmos. Chem. Phys., 22, 561–575, https://doi.org/10.5194/acp-22-561-2022, 2022.

Media contact: Ms. LIN Zheng, jennylin@mail.iap.ac.cn